Zaherite

zaherite

natroalunite

bohmite

hotsonite

Images

Formula: Al12(SO4)5(OH)26.20H2O
Hydrated sulphate
Crystal System: Triclinic
Specific gravity: 2.007 measured, 2.01 calculated
Hardness: 3½
Colour: White to blue-green
Solubility: Dehydrates reversibly at room temperature
Environments

Metamorphic environments
Hydrothermal environments

Localities

At the type locality, the Salt Range, Punjab Province, Pakistan, zaherite is associated with kaolinite, böhmite and and aluminite. Here, zaherite is found both in relatively pure form as veinlets up to 1 cm across that cut massive kaolinite-böhmite rock, and intimately mixed with kaolinite and böhmite in a massive white claystone. Aluminite is also found as veinlets in the vicinity.
Zaherite in fairly pure form was found as densely packed aggregates of extremely small grains (AM 62.1125-1128).
Zaherite from the Salt Range - Image

At the Hotson 6 Mine, Koenabib farm, Khâi-Ma Local Municipality, Namakwa District Municipality, Northern Cape, South Africa, zaherite occurs as veins up to 2 cm wide in close association with natroalunite and hotsonite. It is derived from primary sillimanite but alters to encrustations of hotsonite. The sillimanite occurs as large irregular lenses with size ranging from several metres to hundreds of metres. The zaherite occurs in an arid region with an average rainfall of less than 3 inches per annum. The mode of occurrence suggests that the zaherite is an intermediate mineral in the alteration of natroalunite to hotsonite, the former originally deriving from sillimanite.
Zaheite occurs as sheaves of chalk-white to light bluish green material orientated perpendicular to the walls of the veins (MM 48.131-135).
The aluminous minerals occur in a biotite-sillimanite schist. The alteration products include silicates, oxides, sulphates and sulphides. The prevalent silicates are kaolinite, pyrophyllite, topaz, muscovite and biotite. The oxides are diaspore, rutile, ilmenite and, rarely, corundum. Hydrated oxides are common, particularly goethite. The sulphides and sulphide alteration-products are chalcopyrite, pyrite, covellite, chalcanthite, atacamite and, rarely, brochantite. Sulphates are represented by natroalunite, zaherite and gypsum. The zaherite is associated with hotsonite; rare grains of turquoise were also identified. (CM 23.1.29-34).

Mineral Reactions at the Hotson 6 Mine

Evidence supports a petrogenetic model that involves four chemical reactions that sequentially entailed the transformation of sillimanite to natroalunite, natroalunite to zaherite and zaherite to hotsonite, which is also the order of relative abundance at the Hotson 6 quarry. In a few instances zaherite has formed directly from sillimanite.
The prevalent appearance of natroalunite as the first member of the reaction chain was apparently controlled by the local availability of abundant sodium. All the veins at Koenabib have natroalunite, never alunite, which contrasts with many other comparable occurrences.

(1) sillimanite to natroalunite
3(Al2O3.SiO2) + 2Na+ + 4(SO4)2- + 3H2O + 6H+ = Na2O.3Al2O3.4SO3.6H2O + 3SiO2
A source of sodium is close at hand in the feldspar of the country rock and its alteration products.

(2) Natroalunite to zaherite
2(Na2O.3Al2O3.4SO3.6H2O) + 22H2O = 6Al2O3.5SO3.33H2O + 4Na+ + 3(SO4)2- + 2H+
The transformation merely involves the removal of sodium and some of the sulphate in a hydrous medium. This could easily have been accomplished during a local hydrothermal or weathering event.

(3) Sillimanite to zaherite with no consumption of sodium
6(Al2O3.SiO2) + 5(SO4)2- + 28H2O + 10H+ = 6Al2O3.5SO3.33H2O + 6SiO2 It would seem that this transformation merely requires a very hydrous environment and a source of sulphate, but the fact that the transformation of sillimanite to natroalunite was much more common indicates that a local deficiency of alkalis must be essential as well. This is probably the reason for the relative rarity of zaherite.

(4) Zaherite to hotsonite
11(6Al2O3.5SO3.33H2O) + 12P2O5 = 6(11Al2O3.2P2O5.6SO3.53H2O) + 19(SO4)2- + 26H2O + 38H+ The source of the phosphate essential for the formation of hotsonite is at present obscure. The sulphate required for the formation of natroalunite, zaherite and hotsonite presents no problem because sulphides are ubiquitous in the country rocks as well as in the sillimanite ore. The fairly abundant chalcopyrite is extensively altered to covellite and goethite, and encrustations of chalcanthite and atacamite are common (CM 23.1.29-34).
Zaherite from the Hotson 6 Mine - Image

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