Arsenopyrite

arsenopyrite

galena

sphalerite

chalcopyrite

Images

Formula: FeAsS
Oxidation states: Fe2+As1-S1- (AM 87.1692-1698)
Danaite is a cobalt-bearing variety of arsenopyrite
Sulphide, arsenopyrite group, arsenic-bearing mineral
Crystal System: Monoclinic
Specific gravity: 6.07 measured, 6.18 calculated
Hardness: 5½ to 6
Streak: Black
Colour: Tin white to steel white
Solubility: Arsenopyrite is moderately soluble in nitric acid but insoluble in hydrochloric and sulphuric acids
Common impurities: Ag,Au,Co,Sn,Ni,Sb,Bi,Cu,Pb
Environments:

Pegmatites (sparingly)
Metamorphic environments
Hydrothermal environments

Arsenopyrite is the most common arsenic-bearing mineral. It occurs with tin and tungsten ores in high-temperature hydrothermal deposits, associated with silver and copper ores, galena, sphalerite, pyrite and chalcopyrite. It is frequently associated with gold. It is found in contact metamorphic deposits, and disseminated in limestone.

Localities

At Devil's Peak, Sai Kung District, New Territories, Hong Kong, China, the mineralisation occurred in quartz veins in the contact zone between a granite intrusion and acid volcanic rocks. The mine is now closed, and inaccessible for collecting. Chalcopyrite occurred in the quartz veins with beryl, wolframite, molybdenite, pyrite and arsenopyrite (Hong Kong Minerals (1991). Peng, C J. Hong Kong Urban Council)

The Needle Hill Mine, Needle Hill, Sha Tin District, New Territories, Hong Kong, China, is a tungsten mine, abandoned in 1967. The principal ore is wolframite, and the principal gangue mineral is quartz. Molybdenum also occurs. The mineralisation consists of a series of parallel fissure veins that cut through granite. Wolframite and quartz are the main minerals, but galena, sphalerite, pyrite, molybdenite and fluorite have also been found here (Geological Society of Hong Kong Newsletter 9.3.29-40). The quartz-wolframite veins are of high-temperature hydrothermal formation, and grade into wolframite-bearing pegmatites.
Wolframite is almost always associated with molybdenite. Other associated minerals found occasionally include pyrite, chalcopyrite, arsenopyrite, sphalerite, bismuth, fluorite, topaz and cassiterite
(Hong Kong Minerals (1991). Peng, C J. Hong Kong Urban Council)

At the Huangshaping Mine, Huangshaping Pb-Zn-polymetallic ore field, Guiyang Co., Chenzhou, Hunan, China, arsenopyrite occurs as well formed crystals with a bright metallic lustre, up to 4 mm across, on a dark matrix (AESS).
Arsenopyrite from Huangshaping - Image

At the Yaogangxian Mine, Yaogangxian W-Sn ore field, Yizhang Co., Chenzhou, Hunan, China, arsenopyrite has been found associated with quartz and with fluorite (AESS)
Arsenopyrite from Yaogangxian - Image

At Charcas, Charcas Municipality, San Luis Potosí, Mexico, the primary minerals are sphalerite, galena, chalcopyrite, bornite, tetrahedrite, arsenopyrite, pyrite and silver minerals such as jalpaite, diaphorite and acanthite. In the host rock, as metamorphic or alteration minerals, danburite, datolite, hedenbergite, epidote, chlorite, andradite, actinolite and wollastonite have been reported.
Quartz, calcite and danburite crystallised during the entire life of the systems, throughout the intrusive emplacement, metamorphism, and mineralising events. With depth, both sphalerite and galena decrease while chalcopyrite increases.
Secondary sulphides formed include bornite, covellite, digenite and chalcocite. Native silver, native gold, hematite and goethite were deposited after the sulphides (Minrec 55.6.727-728).
Arsenopyrite is common as part of the ore mineral assemblage and can be expected in all mines. In hand specimens, granular aggregates and larger crystals of stubby, prismatic habit and a brilliant metallic luster can reach 2 cm on edge. Aggregates of stubby, mushroom-shaped crystals are known as large as 20 cm across. Arsenopyrite precipitated earlier than the other sulphides such as sphalerite, chalcopyrite, tetrahedrite and galena. Arsenopyrite has been found deposited over danburite, indicating a very early precipitation of the danburite (Minrec 55.6.732-735).
Arsenopyrite from Charcas - Image

Dry Gill Mine, Caldbeck, Allerdale, Cumbria, England, UK. Arsenic is of widespread occurrence in the vicinity of the mine. Large quantities of arsenopyrite occur in the tungsten-bearing quartz veins in the Carrock tungsten mine, and arsenopyrite also occurs in the lead and baryte mines to the north and east of the Dry Gill mine, sometimes in large quantities. The weathering of arsenopyrite near the surface has given rise to a number of arsenic-bearing alteration products (Minrec 54.5.609-611).

At the Emmons pegmatite, Greenwood, Oxford county, Maine, USA, arsenopyrite may occur in crystals to 2 mm coating löllingite masses. The Emmons pegmatite is an example of a highly evolved boron-lithium-cesium-tantalum enriched pegmatite (R&M 94.6.503).

Alteration

chalcopyrite, arsenopyrite, CO2 and O2 to Fe-tennantite, siderite and sulphur
10CuFeS2 + 4FeAsS + 4CO2 + 8O2 = Cu10Fe2As4S13 + 4Fe(CO3) + 11/2S2
(CM 28.725-738)

chalcopyrite, arsenopyrite and pyrite to Fe-tennantite and troilite
10CuFeS2 + 4FeAsS + FeS2 = Cu10Fe2As4S13 + 13FeS
(CM 28.725-738)

chalcopyrite, arsenopyrite and sulphur to Fe-tennantite and pyrite
10CuFeS2 + 4FeAsS + 13/2S2 = Cu10Fe2As4S13 + 12FeS2
This reaction occurs at a comparatively low temperature (CM 28.725-738).

chalcopyrite, arsenopyrite and sulphur to Fe-tennantite and troilite
l0CuFeS2 + 4FeAsS + l/2S2 = Cu10Fe2As4S13 + l2FeS
(CM 28.725-738)

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